Voronoi diagram of points in the Euclidean plane and its computation is foundational to computational geometry. Polynomial root-finding is the origin of fundamental discoveries in all of mathematics and sciences. There is an intrinsic connection between polynomial root-finding in the complex plane and the approximation of Voronoi cells of its roots through a fundamental family of iteration functions, the ``Basic Family. '' We introduce these connections via the Basic Family properties with respect to Voronoi diagrams, and a corresponding visualization called ``Polynomiography.'' Polynomiography is a medium for art, math, education and science. Then, by making use of properties of the Basic Family we introduce a layering of points within each Voronoi cell of a polynomial root, and prove several novel and nontrivial results. These reveal deeper connections between Voronoi diagrams and polynomial root-finding, and offer applications with respect to ordinary Voronoi diagrams and nontrivial generalizations to be defined. We will pose research problems that may be considered as problems lying at the intersection of computational geometry, polynomial root-finding, discrete dynamical systems and more.